TY - JOUR PY - 2022// TI - Rapid analysis of gunshot residues with single-particle inductively coupled plasma time-of-flight mass spectrometry JO - Forensic science international A1 - Brünjes, Robert A1 - Schüürman, Jan A1 - Kammer, Frank von der A1 - Hofmann, Thilo SP - e111202 EP - e111202 VL - 332 IS - N2 - Gunshot residues (GSRs) from different types of ammunition have been characterized using a new method based on single-particle inductively coupled plasma time-of-flight mass spectrometry (sp-ICP-TOF-MS). This method can analyze thousands of particles per minute enabling rapid sample screening for GSR detection with minimal sample preparation. GSR particles are multi-elemental nanoparticles that are mainly defined by the elements lead, barium, and antimony. Sp-ICP-TOF-MS was also used to identify other elements contained in GSR particles while standard particle classification protocols do not consider the complexities of GSR compositions and can therefore miss out on valuable information. The proposed method can be used to support existing GSR detection methods, especially when lead-free, antimony-free, or tagged ammunition has been used; it also provides a possibility for multi-elemental fingerprinting of GSR particles.
Language: en
LA - en SN - 0379-0738 UR - http://dx.doi.org/10.1016/j.forsciint.2022.111202 ID - ref1 ER -